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Morita, Yasuji; Sasaki, Yuji; Tachimori, Shoichi
Proceedings of International Conference on Back-End of the Fuel Cycle: From Research to Solutions (GLOBAL 2001) (CD-ROM), 7 Pages, 2001/09
no abstracts in English
*; *; *; *
JNC TJ8400 2000-061, 92 Pages, 2000/03
Crystallization procedure is considered to have an advantage in recovering rather pure uranium from contaminated uranium solution and to be applicable for a new reprocessing process. It was confirmed until last year that the reprocessing process with crystallization procedure has a sufficient advantage. But the data for Pu crystallization is very rare. although it is necessary for design of the process with crystallization procedure. In this study, a beaker scale plutonium test was performed in AEA Technology Harwell Laboratory to confirm a behavior of Pu (IV) nitrate under crystallization condition. The results were examined by Mitsubishi Materials Corporation. Test item was a measurement of temperature in case of Pu (IV) nitrate crystallization or freezing of the solution in the following six parameters. (Pu(g/L):200, 100, 50, HNO(m):6, Pu valence:4). (Pu(g/L):200, 100, 50, HNO(m):4, Pu valence:4). Test results were as follows. (1)Pu(IV) nitrate crystallization was not observed even in the case 200g Pu/L and HNO 6M and 4M which were considered to the best condition but crystal of HO and HNO 3HO were observed. (2)Similar results were obtained for the other parameter with lower Pu concentration. (3)We can estimate that Pu(IV) nitrate crystallization will not occurred in the reprocessing process with crystallization procedure. (4)The solubility data of Pu(NO) - HNO-HO system was obtained.
Sugikawa, Susumu; ; ; Nakazaki, Masato; Shirahashi, Koichi; ; *; *; Tsuji, Kenichi*; Tachimori, Shoichi; et al.
JAERI-Tech 97-007, 86 Pages, 1997/03
no abstracts in English
Kakehi, Isao; ; ; ; ; Kajitani, Yukio;
PNC TN9410 97-015, 382 Pages, 1996/12
For the purpose of developing the future nuclear fuel recycle system, the design study of the advanced nuclear fuel recycle system is being conducted. This report describes intermediate accomplishments in the conceptual system study of the advanced nuclear fuel recycle system. Fundamental concepts of this system is the recycle system using molten salt which intend to break through the conventional concepts of purex and pellet fuel system. Contents of studies in this period are as follows, (1)feasibility study of the process by Cd-cathode for nitride fuel (2)application study for the molten salt of low melting point (AlCl+organic salt)(3)research for decladding (advantage of decladding by heat treatment)(4)behavior of FPs in electrorefinning (behavior of iodine and volatile FP chlorides, FPs behavior in chlorination) (5)criticaliy analysis in electrorefiner (6)drawing of off-gas flow diagram (7)drawing of process machinery concept (cathode processor, vibration packing) (8)evaluation for the amounts of the high level radioactive wastes (9)quality of the recycle fuels (FPs contamination of recycle fuel) (10)conceptual study of in-cell handling system (11)meaning of the advanced nuclear fuelrecycle system. The conceptual system study will be completed in describing concepts of the system and discussing issues for the developments.